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no it is not currently possible to assign a keyboard shortcut to any of the JACK Transport modes (None, Slave, Master, Full).

knowing that a similar request has been already filed on github.com issue #37, this might come true in the future, as a brand new Transport > Mode sub-meu on main menu and possibly as a new drop-down tool-button as well.

the effect of this solution--when it gets solved that is--will allow you to assing any keyboard shortcut you want, through Help > Shortcuts... as usual.

cheers